I've gone ahead and reevaluated the list of items for the Booklet, and I've determined 7 items from before that I did not state that are unobtainable and are not present in the VMR Rare Crate. These are:

Code:

CHICKEN_SPAWN_EGG
LARGE_FERN
TALL_GRASS
TURTLE_SPAWN_EGG
VEX_SPAWN_EGG
VILLAGER_SPAWN_EGG
VINDICATOR_SPAWN_EGG

The total number of unobtainables is not 69, but 76.